That would be connecting them in the exact opposite way intended. From the Ultimarc site:
Each LED must have its negative connection (cathode) connected to one of the numbered pins 1-64.
Each LED must also have its positive (anode) connection connected to one of the supply pins marked “+”. Note it does not matter which of the “+” pins you use as they are all connected together on the board.
Unlike buttons, the direction of the current when hooking up LEDs actually matters. This is because they are diodes. If you hook them up incorrectly, at best they won't work. At worst, you could damage them.