I don't think that is quite right, I would expect your monitor has a number of 'locked' refresh rates
That's probably the case. To find it out it's better to use Arcade OSD once you set a modified refresh through Powerstrip, then press 'measure vfreq' and check if the refresh is smooth for the different values. If it's only smooth for values around 60, then the monitor is converting any input signal to 60 Hz. Most 'recent' monitors do this, unfortunately. Some are capable of showing several discrete values, like 57 and 60, and convert everything else.
Anyway, I'd be good to know what card is being used and if it's fully supported by Powerstrip.
You can force syncrefresh for all games by selecting a very high value for the -syncrefresh_tolerance option, such as 10.0. By doing that all games will run smooth but at the wrong speed.